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Phys. , 67, 2344 (1963); Advan. Chfdmutog. 4, 3 (1967). 45. M. ), Steric Effects in Organic Chemistry, Wiley, New York, 1956. 46. H. E. Simmons and J. K. Williams, J. Am. Chem. Soc, 86, 3222 (1964). 47. F. J. Adrian, J. Chem. Phys:, 28, 608 (1958). ;. ~ 48. J. B. Hendrickson, J. Am. Chem. Soc, 83, 4537 (1961). ' •" 49. R. Daudel, R. Le Febvre, and C. Moser, Quantum Chemistry, Methods and Applica­ tions, Wiley (Interscience), New York, 1959. 50. K. Higasi, H. Baba, and A. Rembaum, Quantum Organic Chemistry, Wiley (Inter­ science), New York, 1965.

Type isotherms are assumed typical of sample micelle formation. Unfortun­ ately, these interpretations of isotherm shape represent gross simplifi­ cations, since many different factors contribute to isotherm shape (see below). In at least one instance (32) an adsorption mechanism derived according to the latter scheme has been disproved on other grounds. In two cases where Я-type isotherms have been encountered (33), the presence of a small number of very strong adsorption sites seems much more likely than micelle formation of sample molecules.

S. Petrova, K. D. Shcherbakova, and Ya. I. Yashin, Anal. , 36, 1527 (1964). 36a. A. L. McClellan and H. F. Harnesberger, J. , 23, 577 (1967). V - 37. L. Pauling, The Nature of the Chemical Bond, Cornell" U n r ^ ^ p S f , I t h a c a , N Y . , 1940, Chap. V. Ij- * _ * » / ; / ' ЛЧ. L. R. Snyder and E. R. Fett, J. , 18, 461 ( 1 9 ) 5 5 ) ; ? ¾ ^ 3V. M. J. S. Dewar and P. J. Grisdale, J. Am Chem. Soc, 84* 35$£~{f$62). 40. L. P. Hammet, Physical Organic Chemistry, McGraw-Hill, New York, 1940, 41. H.

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